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Spin physics in 2D van der Waals materials

18 - 19 May 2026 09:00 - 17:00 Apex Grassmarket Hotel Free
Spin physics - lead image

Theo Murphy meeting organised by Professor Hidekazu Kurebayashi, Dr Elton Santos, Professor Cecilia Mattevi, Professor Irina Grigorieva and Professor Konstantin Novoselov FRS.

The dimensionality of materials determines their electronic structures and their fundamental properties. Magnetic order in truly two dimensions has only been discovered in 2017, and since then a plethora of exciting research avenues to understand, manipulate and implement 2D-materials in practical applications has been intensely pursued. This workshop will assemble world-leading scientists to discuss the frontiers of the field.

Programme

The programme, including speaker biographies and abstracts, is available below but please note the programme may be subject to change.

Poster session

There will be a poster session on Monday 18 May 2026. Registered attendees will be invited to submit a proposed poster title and abstract (up to 200 words). Acceptances may be made on a rolling basis so we recommend submitting as soon as possible in case the session becomes full. Submissions made within one month of the meeting may not be included in the programme booklet.

Attending this event

  • Free to attend in-person only
  • When requesting an invitation, please briefly state your expertise and reasons for attending
  • Requests are reviewed by the meeting organisers on a rolling basis. You will receive a link to register if your request has been successful
  • Catering options will be available to purchase upon registering. Participants are responsible for booking their own accommodation. Please do not book accommodation until you have been invited to attend the meeting by the meeting organisers

Please note that scientific meetings hosted by the Royal Society do not necessarily represent a Royal Society position or signify an endorsement of the speakers or content presented.

Enquiries: contact the Scientific Programmes team.

Organisers

  • Professor Hide Kurebayashi

    Professor Hidekazu Kurebayashi

    Hide Kurebayashi is Professor of Condensed Matter Physics and Nanoelectronics at two institutes, UCL and Tohoku University. Before joining UCL, he worked at the University of Cambridge as a JST-PRESTO research fellow in the Cavendish laboratory, where he also completed his PhD in 2010. He leads two experimental research groups in the UK and Japan, working on spintronics and spin dynamics. His recent research interest includes spin-orbit transport in inversion-broken and/or low-dimensional crystals such as van der Waals materials, neuromorphic computing and coherent photon-magnon coupling in nano-systems. For his research, he received the JSPS Prize, Leverhulme Research Fellowship, The Young Scientists’ Award within The Commendation for Science and Technology by the Minister of Education, Culture, Sports, Science and Technology by Japanese government, UCL Future Leader Award, JST-PRESTO Research Fellowship, Darwin College Research Fellowship, Runner-up of the Abdus Salam Prize, ORS and the Nakajima Foundation scholarship.

  • Elton Santos

    Dr Elton Santos

    Dr Santos received his PhD in 2011 from the Danish Technical University with a European Honor. Then, he was awarded a John A Paulson Postdoctoral Fellowship at Harvard University to perform research on energy materials and method developments for functional devices. He moved to Stanford University in 2013 as an assistant staff scientist. Dr Santos moved to the UK in 2015 to start his research group at Queen’s University Belfast (QuB) as a Queen’s Fellow and has taken a leading role on the research of 2D materials and Energy Efficient Processes in QuB. He was promoted to a full Lecturership in 2019. Dr Santos is one of the recipients of the Charles Hatchett 2020 Award for his investigations on energy materials. He moved in 2020 to The University of Edinburgh to hold the position of Reader in Theoretical and Computational Condensed Matter Physics at the School of Physics and Astronomy, and the Higgs Centre for Theoretical Physics. He was elected as a Fellow (FInstP) of the Institute of Physics (IOP) in 2023 and is currently an EPSRC Fellow on energy-efficient quantum magnets.

  • Cecilia Mattevi

    Professor Cecilia Mattevi

    Cecilia is a Professor of Materials Science in the Department of Materials. Her research focuses on the precise synthesis of atomically thin 2D materials with the aim of advancing devices for future computing and achieving carbon neutrality. Cecilia earned a PhD in Materials Science in 2008, conducting her doctoral research at the European Synchrotron Facility, Elettra. She then joined the Materials Science Department at Rutgers University as a postdoctoral researcher, before moving to Imperial College as a Junior Research Fellow. In 2012, Cecilia was appointed as a Lecturer and Royal Society University Research Fellow in the Department of Materials.

  • blank avatar

    Professor Irina Grigorieva

  • Konstantin Novoselov

    Sir Konstantin Novoselov FRS

    Prof Sir Konstantin ‘Kostya’ Novoselov FRS was born in Russia in August 1974. He is best known for isolating graphene at The University of Manchester in 2004, and is an expert in condensed matter physics, mesoscopic physics and nanotechnology. Every year since 2014 Kostya Novoselov is included in the list of the most highly cited researchers in the world. He was awarded the Nobel Prize for Physics in 2010 for his achievements with graphene. His other notable achievements include his work on other 2D materials, their heterostructures, and lately on functional intelligent materials and the application of AI for materials design.

    Kostya is a director of the Institute of Functional Intelligent Materials and holds a position of a Tan Chin Tuan Centennial Professor at the National University of Singapore. He is also part time Langworthy Professor of Physics and the Royal Society Research Professor at The University of Manchester.

    He graduated from the Moscow Institute of Physics and Technology, and undertook his PhD studies at the University of Nijmegen in the Netherlands before moving to The University of Manchester in 2001. Later Professor Novoselov joint the National University of Singapore in 2019. Professor Novoselov has published more than 500 peer-reviewed research papers, including more than 30 in Nature or Science. His h-index is above 155. The paper on the discovery of graphene has more than 60,000 citations, and was included by Nature to the list of 100 most cited papers of all times. He was awarded with numerous prizes, including Nicholas Kurti Prize (2007), International Union of Pure and Applied Science Prize (2008), MIT Technology Review young innovator (2008), Europhysics Prize (2008), Bragg Lecture Prize from the Union of Crystallography (2011), the Kohn Award Lecture (2012), Leverhulme Medal from the Royal Society (2013), Onsager medal (2014), Carbon medal (2016), Dalton medal (2016), Otto Warburg Prize (2019), John von Neumann Professor from the John von Neumann Computer Society (2022), Platinum medal from the Institute of Materials, Minerals and Mining (2024) among many others. He was knighted in the 2012 New Year Honours.

Schedule

Chair

Professor Hide Kurebayashi

Professor Hidekazu Kurebayashi

University College London, UK

08:15-08:20 Welcome by the Royal Society and lead organiser
Professor Hidekazu Kurebayashi

Professor Hidekazu Kurebayashi

University College London, UK

08:20-08:55 Mystery of magnetic exciton in van der Waals antiferromagnet NiPS3

NiPS3 was among the first van der Waals magnets to be exfoliated down to a monolayer in 2016 and remains one of the most intriguing members of this class. Notably, it hosts an exceptionally narrow magnetic exciton below its antiferromagnetic ordering temperature of 155 K. This exciton has been proposed to originate from a transition between two quantum-entangled states: the Zhang-Rice triplet and the Zhang-Rice singlet, and to exhibit remarkable polarisation. Despite extensive experimental confirmation of these observations by multiple groups, the precise microscopic mechanism underlying the exciton formation remains a topic of active debate. In this talk, I will present recent experimental data and theoretical insights that help unravel the nature of this exciton.

Professor Je Geun Park

Professor Je Geun Park

Seoul National University, Korea

08:55-09:10 Discussion
09:10-09:45 Spin and orbital torque induced magnetization dynamics in van der Waals magnets

Exploring spin, orbital, and topological properties of two-dimensional (2D) quantum materials represents a new platform for realising novel quantum and spin-based phenomena and device applications. We showed that the unique band structure and lower crystal symmetries of WTe2 and TaIrTe4 can provide an unconventional spin-polarized current [1] and out-of-plane spin-orbit torque [2] needed for field-free magnetization switching. On the other hand, 2D magnets are promising owing to their tunable magnetic properties. We reported above room temperature 2D magnet-based spin-valve devices in heterostructure with graphene [3,4]. We further utilised such 2D magnets with co-existence of ferromagnetic and anti-ferromagnetic orders with intrinsic exchange bias in the system, giving rise to a canted magnetism [5]. Such canted magnetism of 2D magnets helps in achieving field-free magnetization switching with conventional spin orbit materials such as Pt [5,6]. Combining such 2D quantum materials in van der Waals heterostructures can offer a promising platform for efficient control of magnetization dynamics for non-volatile spin-based memory. Recently, we demonstrated energy-efficient field-free spin-orbit torque (SOT) switching and tunable magnetization dynamics in 2D heterostructure comprising out-of-plane magnet Fe3GaTe2 and topological Weyl semimetal TaIrTe4 [7]. In TaIrTe4/Fe3GaTe2 devices, an energy-efficient and deterministic field-free SOT magnetization switching is achieved at room temperature with a very low current density [7]. These results show that 2D heterostructures provide a promising route to energy-efficient, field-free, and tunable SOT-based spintronic memory devices [8].

References
[1] B Zhao et al, Saroj Dash, Advanced Materials 32, 2000818 (2020)
[2] L Binasal et al, Saroj Dash, Nature Communications 15 (1), 4649 (2024)
[3] B Zhao et al, Saroj Dash, Advanced Materials, 2209113 (2023)
[4] R Ngaloy et al, Saroj Dash, ACS Nano 2024, 18, 7, 5240 (2024)
[5] B Zhao et al, Saroj Dash, Advanced Materials, 2502822 (2025)
[6] B Zhao et al, Saroj Dash, ACS Nano 19, 14, 13817 (2025)
[7] L Pandey et al, Saroj Dash, Nature Communications 16, 8722 (2025)
[8] B Zhao et al, Saroj Dash, https://doi.org/10.48550/arXiv.2602.24046

Professor Saroj Dash

Professor Saroj Dash

Chalmers University of Technology, Sweden

09:45-09:55 Discussion
09:55-10:30 Break
10:30-11:05 Unconventional spin-charge interconversion by twisting van der Waals heterostructures

The low symmetry present in many 2D materials allows the creation of spin polarizations in unconventional directions and enables new fundamental effects and configurations for devices. In this regard, chiral systems are the ultimate expression of broken symmetry, lacking inversion and mirror symmetry. One way to achieve this is by twisting a graphene/transition metal dichalcogenide (TMD) heterostructure. We use twisted graphene/WSe2 to observe spin-charge interconversion arising from Rashba-Edelstein effect (REE) from spins not only perpendicular to the current (conventional configuration), but also parallel to the current (unconventional configuration) [1]. Furthermore, we can tune the twist angle between graphene and WSe2 to control the helicity of the Rashba spin texture, which even changes sign, in excellent agreement with theoretical predictions [2]. Another way to exploit chirality is by placing on graphene a TMD material with a chiral charge density wave (CDW) phase, such as 1T-TaS2, whose commensurability can be controlled with temperature. We have demonstrated that the unconventional REE can be turned on or off by tuning the commensurability of the CDW phase [3]. The disappearance of the unconventional REE arises from the presence of chiral CDW multidomains in the commensurate phase in the heterostructures, where the sign of the unconventional REE is locked to the chirality. The rich interplay between proximity, commensurability, and chirality in the graphene/TMD van der Waals heterostructures opens the path to tailor a plethora of spin-based phenomena in low-dimensional systems.

References
[1] H. Yang, FC et al., Nat. Mater. 23, 1502 (2024)
[2] S. Lee, FC et al. Phys. Rev. B 106, 165420 (2022)
[3] Z. Chi, FC et al., Adv. Mater. 36, 2310768 (2024)

Professor Felix Casanova

Professor Felix Casanova

CIC nanoGUNE, Spain

11:05-11:15 Discussion
11:15-11:50 Complex spin textures and gigantic coercive fields in exfoliated Fe3GaTe2

Here, I will briefly review recent progress in the field of 2D magnets and discuss some of the properties of Fe3GaTe2. This compound is an exfoliable ferromagnet, characterized by a centrosymmetric structure and a Curie temperature exceeding Tc ~ 360 K which, so far, is the highest among 2D magnets. In Fe3GaTe2, several groups report the observation of topologically non-trivial spin textures, such as Néel and Bloch skyrmions well above room temperature which are conventionally understood to require the lack of inversion symmetry, or the Dzyaloshinskii–Moriya interaction among the magnet moments of Fe ions. We argue through detailed structural analysis that such complex spin textures likely result from the local lack of inversion symmetry resulting from intrinsic structural disorder [1]. Our study would provide an explanation for the observation of Néel skyrmions in centrosymmetric systems. Finally, we will discuss preliminary data indicating that the magnetic coercive fields of Fe3GaTe2, for magnetic fields applied along a planar direction, increase by over one order of magnitude upon exfoliation leading to values comparable to those of commercially used hard magnets such as Nd2Fe14B or Sm2Co17 [2]. Therefore, simple exfoliation leads to remarkably large coercivities and magnetic anisotropy at room temperature in a 2D magnet that is critical mineral free, thus opening intriguing prospects for applications.

Professor Luis Balicas

Professor Luis Balicas

Florida State University, US

11:50-12:00 Discussion
12:00-12:35 PT-broken magnetism in orthogonally stacked CrSBr bilayers revealed by magneto-nonlinear optics

The pivotal role of broken PT symmetry in generating novel electromagnetic responses within magnetic systems has gained significant attention in recent years. While considerable efforts have focused on identifying naturally occurring magnets with broken PT symmetry, there has been comparatively little exploration into artificially engineered PT- broken magnetic structures. In this study, we fabricate a bilayer structure by aligning two CrSBr monolayers at a 90° orientation, resulting in an orthogonally stacked configuration. Structurally, this system belongs to the S4 point group, which breaks spatial inversion (P) symmetry. Magnetically, it is expected to break both spatial inversion (P) and time-reversal (T) symmetries, as well as their combined PT symmetry. We employ rotation anisotropy (RA) second harmonic generation (SHG) to probe the temperature and magnetic field dependence of the magnetic phase in the orthogonally stacked CrSBr bilayer, directly revealing its PT-broken nature.

Dr Liuyan Zhao

Dr Liuyan Zhao

University of Michigan, US

12:35-12:45 Discussion

Chair

Elton Santos

Dr Elton Santos

University of Edinburgh, UK

13:45-14:20 Precision quantum measurements on 2D magnets and superconductors

Quantum sensing explores the ultimate limits of measurement sensitivity. When combined with high spatial resolution, it has the potential to provide unprecedented insight into material properties. Spin defects in wide–band-gap semiconductors are among the leading candidates in this field, with systems such as the NV centre in diamond demonstrating an impressive range of applications.

Recently, we used this technique to perform detailed measurements on twisted CrI₃ multilayers [1]. In earlier work, we observed the expected magnetic moiré pattern in twisted double and quadruple layers at small twist angles. Surprisingly, at larger twist angles a new periodic magnetization pattern emerges. We interpret these results in terms of a twist-angle–induced anisotropic exchange interaction [2].

In addition, we probe superconductivity in the two-dimensional superconductor NbSe₂. Measurements of vortices, as well as noise spectroscopy, reveal a rich phase behaviour. We image vortices in the superconducting state and quantify the penetrating magnetic flux [3]. Dephasing measurements of the probe spin provide detailed insight into non-equilibrium phenomena, such as noise generated by quasiparticle fluctuations.

[1] T Song et al. Science 374 (2021) 1140
[2] KC Wong et al. Nature Nano. https://doi.org/10.1038/s41565-025-02103-y (2026)
[3] S Jayaram et al. Phys. Rev. Lett. 135 (2025) 126001

Professor Joerg Wrachtrup

Professor Joerg Wrachtrup

University of Stuttgart, Germany

14:20-14:30 Discussion
14:30-15:00 Magnetic imaging of spin waves and supercurrents using solid-state spins

Spin waves are collective excitations of the spins in magnetic materials. They play an important role in the thermodynamics of magnetic materials and are promising signal carriers in classical and quantum information devices. In this talk, I will introduce spin-wave imaging based on electronic sensor spins in diamond (1) and boron nitride (2) – a magnetic resonance technique that enables studying spin waves underneath optically opaque materials (3). I will then describe experiments on the interaction of spin waves with normal and superconducting metals (4). For normal metals, Ohmic dissipation dominates the diamagnetic response to the stray magnetic fields of the spin waves, leading to spin-wave damping(3). In contrast, the dissipationless diamagnetism of superconductors renormalises the spin-wave dispersion(4), resulting in spin-wave refraction that is tunable by magnetic fields and temperature. The results indicate that superconductors provide opportunities for realising tunable, low-damping spin-wave optical devices that could be used for microwave-control in classical or quantum circuits.

1. I Bertelli et al., Magnetic resonance imaging of spin-wave transport and interference in a magnetic insulator. Sci. Adv. 6, eabd3556 (2020)
2. S Mañas-Valero et al., Isofrequency spin-wave imaging using color center magnetometry for magnon spintronics. Nat. Commun. 17, 379 (2025)
3. I Bertelli et al., Imaging Spin‐Wave Damping Underneath Metals Using Electron Spins in Diamond. Adv. Quantum Technol. 4, 2100094 (2021)
4. M Borst et al., Observation and control of hybrid spin-wave–Meissner-current transport modes. Science. 382, 430–434 (2023)

Professor Toeno van der Sar

Professor Toeno van der Sar

Delft University of Technology, The Netherlands

15:00-15:10 Discussion
15:10-15:30 Break
15:30-16:05 Single optically active spin defects in hexagonal boron nitride for quantum technologies

Quantum networks and sensing require solid-state spin-photon interfaces that combine single-photon generation and long-lived spin coherence with scalable device integration, ideally at ambient conditions. Despite rapid progress reported across several bulk materials systems, those possessing quantum coherent single spins at room temperature remain extremely rare. Recently, it has been discovered that the 2D material hexagonal boron nitride (hBN) also hosts atomic scale defects with optically addressable spins. In this talk, I will present a single photon emitting carbon-related defect in hBN that has a spin-triplet ground state which can be coherent controlled under ambient conditions [1][2]. I will reveal that the spin coherence is governed predominantly by coupling to only a few proximal nuclei and is prolonged by decoupling protocols. In addition, I will prevent magnetic field-dependent magnetic resonance and photoluminescence data that enables us to probe the defect’s electronic structure and suitability for nanoscale magnetometry [3].

[1] Stern, H.L., M. Gilardoni, C., Gu, Q. et al. A quantum coherent spin in hexagonal boron nitride at ambient conditions. Nat. Mater. 23, 1379–1385 (2024)

[2] Stern, H.L., Gu, Q., Jarman, J. et al. Room-temperature optically detected magnetic resonance of single defects in hexagonal boron nitride. Nat Commun 13, 618 (2022)

[3] Gilardoni, C. M., Eizagirre Barker, S., Curtin, C. L., Fraser, S. A., Powell, O. F.J., Lewis, D. K., Deng, X., Ramsay, A. J., Li, C., Aharonovich, I., Tan, H. H., Atatüre, M. and Stern, H. L.. arXiv.:2408.10348 (2024)

Dr Hannah Stern

Dr Hannah Stern

University of Oxford, UK

16:05-16:15 Discussion
16:15-16:50 Imaging the sub-moiré potential landscape using an Atomic Single Electron

Electrons in solids owe their properties to the periodic potential landscapes they experience. The advent of moiré lattices has revolutionized our ability to engineer such landscapes on nanometer scales, leading to numerous groundbreaking discoveries. Despite this progress, direct imaging of these electrostatic potential landscapes remains elusive. Here, we introduce the Atomic Single Electron Transistor (SET), a novel scanning probe that uses a single atomic defect in a van der Waals (vdW) material as an ultrasensitive, high-resolution potential sensor. Built upon the quantum twisting microscope (QTM) platform, this probe leverages the QTM’s capability to form a pristine, scannable 2D interface between vdW heterostructures. Using the Atomic SET, we present the first direct images of the electrostatic potential in a canonical moiré interface: graphene aligned to hexagonal boron nitride. This potential exhibits an approximate C_6 symmetry, minimal dependence on carrier density, and a substantial magnitude of ~60 mV even in the absence of carriers. Theory indicates that this symmetry arises from a delicate interplay of physical mechanisms with competing symmetries. Intriguingly, the measured magnitude significantly exceeds theoretical predictions, suggesting that current understanding may be incomplete. With 1 nm spatial resolution and sensitivity to potentials generated by only a few millionths of an electron’s charge, the Atomic SET enables ultrasensitive imaging of charge order and thermodynamic properties across a wide range of quantum phenomena, including symmetry-broken phases, quantum crystals, vortex charges, and fractionalized quasiparticles.

Dr Dahlia Klein

Dr Dahlia Klein

University of Chicago, US

16:50-17:00 Discussion
16:50-17:00 Close

Chair

Cecilia Mattevi

Professor Cecilia Mattevi

Imperial College London, UK

08:20-08:55 Tuning magnetic order in epitaxially grown van der Waals magnets: From 2D-XY systems to high-Tc magnets driven by self-intercalation

I will discuss how the bottom-up growth of van der Waals magnets by molecular beam epitaxy (MBE) promotes favourable conditions to stabilize specific magnetic behaviour which has remained elusive on studies with exfoliated bulk crystal flakes – such as 2D-XY anisotropy and enhancement of magnetic exchange driven by self-intercalation. First, I will focus on the successful van-der-Waals epitaxy of a CrCl3 monolayer grown on Graphene/6H-SiC(0001), revealing intrinsic ferromagnetic order with easy-plane anisotropy and a 2D-XY magnetic universality class [1].  This constitutes the first realization of a Berezinskii-Kosterlitz-Thouless (BKT) transition in a 2D magnet, with important implications in the stabilization of topological spin textures with in-plane winding, i.e. merons. The important role of the van der Waals substrate interaction and the underlying crystal symmetry to achieve this rather unsual magnetic behaviour will be discussed, thereby highlighting routes on how to control the anisotropy of 2D magnets via growth and substrate engineering.

Further peculiarities of MBE-grown van der Waals magnets, such as an increase of the Curie Temperature driven by self-intercalation [2], will be shown in the prototypical layered magnet Fe5GeTe2. The epitaxial films exhibit ferromagnetic ordering up to 375 K, concomitant with a sizable Fe occupation within the van der Waals gaps. Supported by first-principles calculations, we infer that the higher magnetic ordering temperature results from an increased exchange interaction among the Fe5GeTe2 layers mediated by Fe within the vdW gaps. Our findings establish self-intercalation during epitaxial growth as an efficient mechanism to achieve high-temperature magnetism in a broad class of van der Waals materials.

[1]  Bedoya-Pinto, et.al. Intrinsic 2D-XY ferromagnetism in a van der Waals monolayer. Science 374 (6567), 616-620 (2021)
[2]  Silinskas, et. al. Self-intercalation as origin of high-temperature ferromagnetism in epitaxially grown Fe5GeTe2 thin films. Physical Review Letters 133, 256702 (2024)

Dr Amilcar Bedoya-Pinto

Dr Amilcar Bedoya-Pinto

University of Valencia, Spain

08:55-09:10 Discussion
09:10-09:45 Electronic and magnetic structure in epitaxial van der Waals heterostructures

The transition-metal chalcogenides include some of the most important and ubiquitous families of 2D materials. Their van der Waals nature allows for the ready isolation of single layers, while they host an exceptional variety of electronic and magnetic states which can in principle be readily tuned by combining different 2D layers in van der Waals heterostructures [1]. Growth via molecular-beam epitaxy (MBE) should be a premier route to achieve this, but efforts have been hampered by non-uniform layer coverage [2], unfavourable growth morphologies, the presence of significant rotational disorder, and limited growth windows and growth rates. I will discuss how a dramatic enhancement in quality of MBE-grown 2D materials can be achieved by simple substrate pre-treatments which dramatically enhance the epilayer nucleation, in turn facilitating a desired layer-by-layer growth mode [3,4]. I will show how this leads to an expanded growth window for metastable materials, allowing, for example the selective stabilisation of high-coverage CrTe2 and Cr2+εTe3 epitaxial monolayers [5]. This, in turn, opens the door to spectroscopic investigations of their magnetic and electronic structures [5,6], and enables their use to induce magnetism in neighbouring 2D layers via proximity coupling in van der Waals heterostructures [7].

[1] Chhowalla et al., Nat. Chem. 5 (2013)
[2] Rajan et al., Phys. Rev. Mater. 4 (2020) 014003
[3] Rajan et al., Adv. Mater. 36 (2024) 2402254
[4] Rajan et al., APL Mater. 13 (2025) 081123
[5] Kushwaha et al., npj Quantum Materials 10 (2025) 50
[6] Armitage et al., Phys. Rev. B in press (arXiv:2505.07942 (2025))
[7] Kushwaha, Rajan et al.in preparation

Professor Phil King

Professor Phil King

University of St Andrews, UK

09:45-09:55 Discussion
09:55-10:30 Break
10:30-11:05 Probing magnetic excitations in 2D quantum magnets: topology with magneto-Raman spectroscopy

The topology of magnetic excitations is an exciting new field of study that merges two mature subjects in condensed matter physics that offers a new way of understanding quantum magnets. Long lifetime, surface localisation, and backscattering protection are some of the characteristics of topologically non-trivial magnetic excitations. Such properties make them attractive for potential applications in spintronic and quantum sensing devices. Experimentally identifying and verifying topological magnetic excitations has been challenging because there is not a single experimental method that can do so.

In this talk I will briefly introduce the theory of topological magnons and present two examples, one a quasi-2D magnet [1,2] and the other a non-coplanar antiferromagnet [3], of how use magneto-Raman spectroscopy in combination with inelastic neutron scattering results to identify these quasiparticles. Our conclusions are enabled by the combination of topological theory, inelastic neutron scattering, and the experimental suite at NIST of unique magneto-Raman spectroscopic instrumentation that enables diffraction-limited, spatially- and polarization-resolved Raman measurements while simultaneously varying the temperature (1.6 K to 400 K), laser wavelength (tunability from visible to near-infrared), and magnetic field (up to 9 T). Time-permitting, I will summarise results on additional 2D van der Waals antiferromagnets [4,5,6] also studied at NIST.

[1] Yufei Li, Thuc T Mai, et al. Phys. Rev. B. 109, 184436 (2024)
[2] Thuc T Mai, Yufei Li, et al. Phys. Rev. B. 111, 104419 (2025)
[3] Ahmed E Fahmy, et al. ArXiv:2512.18534. In review
[4] Thuc T Mai, et al. Sci. Adv. 7, eabj3106 (2021)
[5] Amber McCreary, et al. Nat. Comm. 11, 3879 (2020)
[6] Amber McCreary, et al. Phys. Rev. B. 101, 064416 (2020)

Dr Rolando Valdés Aguilar

Dr Rolando Valdés Aguilar

National Institute of Standards and Technology, US

11:05-11:15 Discussion
11:15-11:50 All-optical control of spins in van der Waals magnets

Recently discovered two-dimensional (2D) van der Waals (vdW) magnets offer new opportunities for controlling magnetism via mechanisms such as strain, voltage, and twistronics. Ultrafast laser pulses provide the fastest means of manipulating magnetic properties, yet their effects on spins in 2D magnets remain largely unexplored. In this talk, I will discuss all-optical control of the 2D vdW ferromagnets CrI3 [1] and Cr2Ge2Te6 [2,3].

Our research shows that integrating a thin CrI3 flake with a monolayer of transition metal dichalcogenide WSe2 enables helicity-dependent all-optical switching (AOS) down to a single laser pulse [1]. I will also demonstrate that optical pumping can lead to formation of various spin textures, including reversible transformations between stripe and bubble/skyrmion phases in Cr2Ge2Te6 [2]. Finally, I will discuss thickness dependent remagnetisation dynamics in Cr2Ge2Te6 observed via time-resolved beam-scanning Kerr microscopy [3]. Our findings reveal that reducing the thickness of the 2D magnet enhances heat dissipation to the substrate, significantly shortening the magnetisation recovery time from several nanoseconds to a few hundred picoseconds.

[1] M Dąbrowski, et al. Nat. Commun. 13, 5976, (2022)
[2] M Khela, M Dąbrowski, et al. Nat. Commun. 14, 1378 (2023)
[3] M Dąbrowski, et al. Nat. Commun. 16, 2797, (2025)

Dr Maciej Dabrowski

Dr Maciej Dabrowski

University of Exeter, UK

11:50-12:00 Discussion
12:00-12:35 Growing insights: the role of in situ diffraction in the formation of single-crystalline quantum materials

Understanding how quantum materials form at the atomic scale is essential for unlocking their extraordinary properties. Single-crystalline phases, especially rare-earth intermetallics, kagome lattices, and germanides, offer a rich platform for exploring strongly correlated electron systems, topological metals, and emergent magnetic phenomena. Achieving these crystals often relies on flux growth, a powerful technique that enables slow, controlled crystallization from a molten medium. Yet, the mechanisms governing nucleation, phase competition, and structural evolution during flux growth remain largely hidden.

Our research employs in situ diffraction as a real-time probe to capture these dynamics, revealing how subtle van der Waals interactions and heterostructure subunits, distinct structural blocks that stack and interlink, guide the assembly of layered architectures. By visualizing growth pathways as they unfold, we identify critical conditions for stabilizing kagome frameworks and complex motifs that host exotic states such as Dirac fermions and unconventional magnetism. Combining predictive design with flux growth and real-time structural insight transforms synthesis into a science of controlled complexity. In this presentation, I will demonstrate how in situ diffraction enables rational strategies for growing rare-earth intermetallic kagome and germanide systems with unprecedented precision, paving the way for quantum functionalities once considered out of reach.

Professor Julia Chan

Professor Julia Chan

Baylor University, US

12:35-12:45 Discussion

13:45-14:20 Surface acoustic wave–driven magnon–phonon coupling in layered van der Waals antiferromagnet CrCl₃

Antiferromagnets offer ultrafast spin dynamics, robustness against stray fields, and rich opportunities for spintronic functionality, yet probing their internal magnetic excitations remains challenging due to their vanishing net magnetization. In this work, we demonstrate a direct mechanical route to excite and detect spin dynamics in a crystalline van der Waals antiferromagnet, chromium trichloride (CrCl₃), by employing surface acoustic waves (SAWs). Using piezoelectric LiNbO₃ substrates with interdigital transducers, we observe clear signatures of acoustic and optical spin-wave resonances driven by SAW irradiation in the gigahertz range. The coupling strength and resonance conditions exhibit pronounced dependencies on temperature and magnetic-field orientation, revealing a sensitivity to minute uniaxial anisotropy fields on the order of millitesla. A theoretical model extending conventional ferromagnetic SAW–magnon coupling formalism to antiferromagnetic systems quantitatively reproduces the experimental behaviour. These findings establish surface acoustic waves as a highly sensitive, non-invasive probe of magnetoelastic interactions in low-dimensional magnets. The demonstrated acoustic antiferromagnetic resonance provides a key platform for exploring dynamic spin–lattice coupling, strain-tunable magnetism, and coherent magnon–phonon control in van der Waals heterostructures.

Professor Yoshichika Otani

Professor Yoshichika Otani

University of Tokyo, Japan

14:20-14:30 Discussion
14:30-15:00 Density Functional Bogoliubov-de Gennes theory for superconductors

Superconductors are materials that conduct electrical current without resistance below a critical temperature due to a mechanism that pairs electrons into coherent quantum states. Their unique properties enable transformative technologies ranging from particle accelerator magnets and MRI scanners to emerging quantum technologies such as qubits and ultrasensitive detectors. At present, all large-scale and commercial applications rely on conventional superconductors, in which the pairing mechanism is well understood and described within the Bardeen–Cooper–Schrieffer (BCS) framework. However, these materials operate only at extremely low temperatures, typically between 1 and 10 K, requiring bulky and energetically expensive cryogenic infrastructures. This not only limits widespread deployment but also raises significant sustainability concerns and hinders miniaturization and portability. High-temperature superconductors offer a possible solution. However, the microscopic mechanism driving high-temperature superconductivity goes beyond BCS theory and remains unknown. Without a predictive understanding of the pairing mechanism, it is impossible to rationally design new superconducting materials with elevated critical temperatures beyond known families.

With my group, we target this long-term ambitious project. We developed a theoretical framework and code implementation for the simultaneous solution of the superconducting (Bogoliubov-de Gennes, BdG) and electronic (Density Functional Theory, DFT) problems. Our method, SIESTA-BdG, is implemented in SIESTA, a first-principles DFT code for material simulations. Our unified approach describes both conventional and unconventional superconducting phases, and enables a description of inhomogeneous superconductors, heterostructures, and proximity induced superconductivity. We demonstrate the validity, accuracy, and efficiency of SIESTA-BdG by computing physically relevant quantities (superconducting charge density, band structure, superconducting gap features, density of states) for conventional singlet (Nb, Pb) and unconventional (FeSe) superconductors. We find excellent agreement with experiments. SIESTA-BdG forms the basis for modeling quantum transport in superconducting devices, and to bridge DFT with Dynamical Mean-Field Theory (DMFT) to model high-temperature superconductivity in strongly correlated electron systems.

Professor Zeila Zanolli

Professor Zeila Zanolli

Utrecht University, Netherlands

15:00-15:10 Discussion
15:10-15:30 Break
15:30-16:05 Spin torque and energy harvesting devices based on 2D materials

The non-volatile spin-torque memory is emerging as a key enabler of low-power technologies, which are expected to spread across large markets, from embedded memories to the Internet of Things. We present our perspective on spin-orbit torque (SOT) device applications using the emerging family of quantum van der Waals materials. Previous proposals for field-free SOT switching of perpendicular magnetic anisotropy (PMA) require either additional magnetic layers or structural engineering, which not only complicate the fabrication process but also impede the scalability and stability. Exploiting the out-of-plane damping-like torque could be a solution for this challenge. Here we experimentally demonstrate field-free switching of PMA CoFeB at room temperature utilising out-of-plane (z) spins from Weyl semimetals, TaIrTe4 and PtTe2/WTe2. Both in-plane and out-of-plane spin Hall conductivities are almost one order of magnitude larger than those from other 2D materials and antiferromagnets, leading to substantial switching power reduction. Notably, the highest out-of-plane spin Hall conductivity in PtTe2/WTe2 bilayers is attributed to spin-to-spin conversion in WTe2 induced by crystal asymmetry. Finally, we show a proof of concept RF energy harvesting device using the nonlinear Hall effect (NLHE) induced by crystal symmetry breaking. Our works open a door to realising room-temperature applications based on 2D materials.

Dr Hyunsoo Yang

Dr Hyunsoo Yang

National University of Singapore, Singapore

16:05-16:15 Discussion
16:15-16:50 Quantum sensing of Moiré magnetism

Moiré magnetism featured by stacking engineered atomic registry and lattice interactions has recently emerged as an appealing quantum state of matter at the forefront of condensed matter physics research. Nanoscale imaging of moiré magnets is highly desirable and serves as a prerequisite to investigate a broad range of intriguing physics underlying the interplay between topology, electronic correlations, and unconventional magnetism. In this talk, I will present our recent work on using nitrogen-vacancy (NV) centres to perform nanoscale quantum sensing and imaging of magnetic domains and spin fluctuations in twisted double trilayer (tDT) chromium triiodide CrI3. We show that intrinsic moiré domains of opposite magnetizations appear over arrays of moiré supercells in low-twist-angle tDT CrI3 [1]. In addition, spin fluctuations measured in tDT CrI3 reveal two distinct magnetic phase transitions with separate critical temperatures within a moiré supercell [2]. Our results enrich the current understanding of exotic magnetic phases sustained by moiré magnetism and highlight the opportunities provided by quantum spin sensors in probing microscopic spin related phenomena on two-dimensional flatland. Lastly, I will extend my discussion to briefly present our ongoing efforts on exploring next-generation van der Waals quantum sensing technologies using color centres beyond NVs [3, 4, 5].

References:
1. M Huang et al., Nat. Commun. 14, 5259 (2023)
2. S Li et al., Nat. Commun. 15, 5712 (2024)
3. M Huang et al., Nat. Commun. 13, 5369 (2022)
4. J Zhou et al., Sci. Adv. 10, eadk8495 (2024)
5. X Zhang et al., arXiv:2502.04561 (2025)

Professor Chunhui (Rita) Du

Professor Chunhui (Rita) Du

Georgia Institute of Technology, US

16:50-17:00 Discussion
17:00-00:00 Close